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Physics

Enhanced superconductivity and mixed-dimensional behaviour in infinite-layer samarium nickelate thin films

Rare-earth infinite-layer nickelates are emerging unconventional superconductors, with materials synthesis largely limited to early lanthanide compounds.

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1 min read

Imagine a world where electricity can flow without resistance, not just in wires but in materials themselves. Researchers have made a breakthrough in creating superconducting materials that were previously thought impossible to synthesize. Yang M and their team successfully created phase-pure samarium-based nickelate thin films on a specific substrate, marking the first demonstration of Sm1-xSrxNiO2 - a material that was once considered too complex to produce.

The journey began by carefully crafting these materials with precise control over their composition. By varying the concentration of samarium and strontium, the team found a sweet spot where superconducting transitions could occur at surprisingly high temperatures - up to 32.5 K. But what's truly remarkable is how the material behaves when you apply different forces or angles: it reveals a unique blend of two-dimensional and three-dimensional superconductivity.

This breakthrough not only expands our understanding of superconductors but also offers new avenues for designing materials with enhanced properties. By manipulating the structure of these rare-earth nickelates, researchers can potentially create even more powerful superconducting materials that could transform industries from energy to transportation. This discovery is a testament to human ingenuity and the power of scientific collaboration, reminding us that even the most seemingly insurmountable challenges can be overcome with careful observation, precise control, and creativity.

The people behind the work

  • Yang M et al.

    Author

    Published in Nature communications

Source: Nature communications

Sources & Verification

Every statement in this story is drawn from the facts below. Each is linked to a primary or reputable source — follow any citation to check it for yourself.

  1. Rare-earth infinite-layer nickelates are emerging unconventional superconductors, with materials synthesis largely limited to early lanthanide compounds. Nature communications
  2. Here, we report phase-pure samarium-based nickelate thin films on (LaAlO 3 ) 0.3 (Sr 2 TaAlO 6 ) 0.7 (001) substrates, including the first demonstration of Sm 1-x Sr x NiO 2 . Nature communications
  3. Co-doped compounds achieve a record-small c-axis parameter (3.26 Å) and superconducting transitions up to 32.5 K, revealing a clear correlation between decreasing c-axis parameter and increasing critical temperature across different rare-earth systems. Nature communications
  4. Angle-dependent magnetoresistance shows a hybrid 2D/3D superconductivity with enhanced rare-earth 5d-Ni 3 d orbital coupling, confirmed by resonant inelastic X-ray scattering. Nature communications
  5. In addition, increasing Eu concentration drives a shift toward 3D superconductivity, and Eu-containing samples exhibit distinctive negative magnetoresistance even in the superconducting state. Nature communications
  6. These findings advocate clear materials design principles for higher transition temperatures and exotic physics in infinite-layer nickelate superconductors through structural engineering of the rare-earth site. Nature communications

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